Ipzz-266

The convergence of ionic liquids (ILs) and conjugated polymers (CPs) has opened a promising route toward multifunctional materials that simultaneously transport ions and electrons. ILs possess negligible vapor pressure, high ionic conductivity, and wide electrochemical windows, whereas CPs such as polythiophene, polypyrrole, and poly(3,4‑ethylenedioxythiophene) (PEDOT) provide delocalized π‑electron pathways for electronic conduction. Merging these two families into a single polymeric scaffold—poly(ionic‑liquid) (PIL) composites—has demonstrated enhanced charge storage, mechanical robustness, and processability (see Ref. [1‑4]).

Despite rapid progress, most reported PIL‑CP hybrids suffer from either (i) insufficient electronic conductivity due to excessive ionic side‑chains that disrupt conjugation, or (ii) limited ion transport because the conjugated backbone hinders ion mobility. A rational molecular design that balances these competing demands is therefore required. In this work we introduce IPZZ‑266, a modular PIL where imidazolium‑based ionic liquid monomers are covalently grafted onto a poly(3‑hexylthiophene) (P3HT) backbone through a short, flexible ether linker. The resulting architecture preserves the planarity of the thiophene units, enabling effective π‑π stacking, while the densely packed ionic moieties furnish continuous ion‑transport channels. IPZZ-266

The objectives of this study are:

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Poly(ionic‑liquid); conjugated polymer; IPZZ‑266; ionic conductivity; electronic conductivity; flexible supercapacitor; strain sensor.